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Black materials are often the most difficult to identify, but a rock hound friend of mine identified the cross as Labrodite (also spelled "Labradorite").
I cannot prove that, so I priced it as glass, although I am not sure it makes much difference either way. It is a really lovely and simple cross in excellent vintage condition.
The last photo shows how this would look on a black glass beaded chain, just as one idea, and it would also look good on a silver chain. View
All items in excellent vintage condition unless otherwise noted.